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Scientific Articles - PTR-MS Bibliography

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[Laat2001] de Laat, ATJ., JA. de Gouw, J. Lelieveld, and A. Hansel, "Model analysis of trace gas measurements and pollution impact during INDOEX", Journal of Geophysical Research: Atmospheres (1984–2012), vol. 106, no. D22: Wiley Online Library, pp. 28469–28480, 2001.
An analysis of acetone (CH3COCH3) and acetonitrile (CH3CN) measurements, performed during the Indian Ocean Experiment (INDOEX), using a chemistry general circulation model is presented. A comparison with measurements indicates that the model simulates realistic CO and acetone distributions, except toward the Indian west coast near the surface. The latter may be related to a sea breeze circulation at the Indian west coast, which is not resolved by the model. A comparison of the measured and modeled correlation between CO and acetone indicates the presence of a background marine acetone source. A model sensitivity study suggests a global marine emission strength of 15-20 Tg acetone yr-1, which is a significant contribution to the estimated global acetone source of 56 (37-80) Tg acetone yr-1. The comparison of measured and modeled CO-acetonitrile correlation from surface measurements indicates that a model sink of acetonitrile in the marine boundary layer is missing. A model sensitivity study suggests that this could be dry deposition (deposition velocity estimate: 0.01-0.05 cms-1) on the ocean surface. A comparison of measured and modeled tropospheric acetonitrile indicates that the model overestimates the free tropospheric acetonitrile mixing ratios up to a factor of 3, which points to a missing free tropospheric sink of acetonitrile in the model. A possible explanation may be stratospheric loss and subsequent stratosphere-troposphere exchange, which was not included in the model.

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Selected PTR-MS related Reviews

F. Biasioli, C. Yeretzian, F. Gasperi, T. D. Märk: PTR-MS monitoring of VOCs and BVOCs in food science and technology, Trends in Analytical Chemistry 30 (7) (2011).

J. de Gouw, C. Warneke, T. Karl, G. Eerdekens, C. van der Veen, R. Fall: Measurement of Volatile Organic Compounds in the Earth's Atmosphere using Proton-Transfer-Reaction Mass Spectrometry. Mass Spectrometry Reviews, 26 (2007), 223-257.

W. Lindinger, A. Hansel, A. Jordan: Proton-transfer-reaction mass spectrometry (PTR–MS): on-line monitoring of volatile organic compounds at pptv levels, Chem. Soc. Rev. 27 (1998), 347-375.


Lists with PTR-MS relevant publications of the University of Innsbruck can be found here: Atmospheric and indoor air chemistry, IMR, Environmental Physics and Nano-Bio-Physics


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